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Investigations of Ra^+ properties to test possibilities of new optical frequency standards

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arxiv 0706.1705 v3 pith:FSUNLXQC submitted 2007-06-12 physics.atom-ph physics.optics

Investigations of Ra^+ properties to test possibilities of new optical frequency standards

classification physics.atom-ph physics.optics
keywords frequencyopticalquadrupolestatesstudiesappropriateatomiccalculations
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The present work tests the suitability of the narrow transitions $7s \ ^2S_{1/2} \to 6d ^2D_{3/2}$ and $7s ^2S_{1/2} \to 6d ^2D_{5/2}$ in Ra$^+$ for optical frequency standard studies. Our calculations of the lifetimes of the metastable $6d$ states using the relativistic coupled-cluster theory suggest that they are sufficiently long for Ra$^+$ to be considered as a potential candidate for an atomic clock. This is further corroborated by our studies of the hyperfine interactions, dipole and quadrupole polarizabilities and quadrupole moments of the appropriate states of this system.

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