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arxiv 2009.13966 v2 pith:3DDNDCJM submitted 2020-09-29 cond-mat.mtrl-sci cond-mat.mes-hall

Influence of molecular beam effusion cell quality on optical and electrical properties of quantum dots and quantum wells

classification cond-mat.mtrl-sci cond-mat.mes-hall
keywords quantumcapacitance-voltagecelldotsaluminumanomaliesbeamcharges
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Quantum dot heterostructures with excellent low-noise properties became possible with high purity materials recently. We present a study on molecular beam epitaxy grown quantum wells and quantum dots with a contaminated aluminum evaporation cell, which introduced a high amount of impurities, perceivable in anomalies in optical and electrical measurements. We describe a way of addressing this problem and find that reconditioning the aluminum cell by overheating can lead to a full recovery of the anomalies in photoluminescence and capacitance-voltage measurements, leading to excellent low noise heterostructures. Furthermore, we propose a method to sense photo-induced trap charges using capacitance-voltage spectroscopy on self-assembled quantum dots. Excitation energy-dependent ionization of defect centers leads to shifts in capacitance-voltage spectra which can be used to determine the charge density of photo-induced trap charges via 1D band structure simulations. This method can be performed on frequently used quantum dot diode structures.

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