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Fermion-boson many-body interplay in a frustrated kagome paramagnet

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arxiv 2007.00519 v1 pith:JNF5V6ZL submitted 2020-07-01 cond-mat.mtrl-sci cond-mat.str-el

Fermion-boson many-body interplay in a frustrated kagome paramagnet

classification cond-mat.mtrl-sci cond-mat.str-el
keywords kagomebosonicfermionicflat-bandmodefrustratedcouplingelectronic
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Kagome-net, appearing in areas of fundamental physics, materials, photonic and cold-atom systems, hosts frustrated fermionic and bosonic excitations. However, it is extremely rare to find a system to study both fermionic and bosonic modes to gain insights into their many-body interplay. Here we use state-of-the-art scanning tunneling microscopy and spectroscopy to discover unusual electronic coupling to flat-band phonons in a layered kagome paramagnet. Our results reveal the kagome structure with unprecedented atomic resolution and observe the striking bosonic mode interacting with dispersive kagome electrons near the Fermi surface. At this mode energy, the fermionic quasi-particle dispersion exhibits a pronounced renormalization, signaling a giant coupling to bosons. Through a combination of self-energy analysis, first-principles calculation, and a lattice vibration model, we present evidence that this mode arises from the geometrically frustrated phonon flat-band, which is the lattice analog of kagome electron flat-band. Our findings provide the first example of kagome bosonic mode (flat-band phonon) in electronic excitations and its strong interaction with fermionic degrees of freedom in kagome-net materials.

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