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Sustained phase separation and spin glass in Co-doped K_(x)Fe_(2-y)Se₂ single crystals

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arxiv 1604.03545 v1 pith:7MATYFKV submitted 2016-04-12 cond-mat.supr-con cond-mat.mtrl-scicond-mat.str-el

Sustained phase separation and spin glass in Co-doped K_(x)Fe_(2-y)Se₂ single crystals

classification cond-mat.supr-con cond-mat.mtrl-scicond-mat.str-el
keywords phasearrangementglassspinsuperconductingconcentrationsmetallicsemiconducting
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We present Co substitution effects in K$_{x}$Fe$_{2-y-z}$Co$_{z}$Se$_{2}$ (0.06 $\leq$ $z$ $\leq$ 1.73) single crystal alloys. By 3.5\% of Co doping superconductivity is suppressed whereas phase separation of semiconducting K$_{2}$Fe$_{4}$Se$_{5}$ and superconducting/metallic K$_{x}$Fe$_{2}$Se$_{2}$ is still present. We show that the arrangement and distribution of superconducting phase (stripe phase) is connected with the arrangement of K, Fe and Co atoms. Semiconducting spin glass is found in proximity to superconducting state, persisting for large Co concentrations. At high Co concentrations ferromagnetic metallic state emerges above the spin glass. This is coincident with changes of the unit cell, arrangement and connectivity of stripe conducting phase.

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