THz response and colossal Kerr rotation from the surface states of the topological insulator Bi₂Se₃

Ordered states of matter are typically categorized by their broken symmetries. With the ordering of spins in a ferromagnet or the freezing of a liquid into a solid, the loss of symmetry distinguishes the ordered state from the disordered one. In contrast, topological states are distinguished by specific \textit{topological} properties that are encoded in their quantum mechanical wavefunctions. Frequently, a consequence of these properties is that there are robust "topologically protected" states on the sample's boundaries. The edge states of the quantum Hall effect (QHE) are the classic example. In the last few years, it was realized that another class of such topological matter may exist in 3D band insulators with large spin-orbit interaction. These so-called topological insulators are predicted to host robust surface states, which exhibit a number of interesting properties including spin helicity, immunity to back-scattering, and weak \textit{anti}--localization. There are predictions of a number of unusual phenomena associated with these surface states, including a proximity-effect-induced exotic superconducting state with Majorana fermions bound to a vortex and an `axion' electromagnetic response, and proposals for applications, such as their use in terahertz devices. In this Letter we report the observation of an unprecedentedly large rotation of the polarization plane of linearly polarized light reflected from thin films of the topological insulator Bi$_2$Se$_3$ in magnetic fields. This Kerr rotation can be as large as 65$^\circ$ and is due almost entirely to the surface states. Our results are evidence for the intrinsic response of the topologically protected surface states and provide a benchmark for the large magneto-electric effect predicted for these materials.