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Direct Evidence for the Dirac-Cone Topological Surface States in Ternary Chalcogenide TlBiSe2

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arxiv 1006.2437 v2 pith:JJM23D4W submitted 2010-06-12 cond-mat.mes-hall cond-mat.str-el

Direct Evidence for the Dirac-Cone Topological Surface States in Ternary Chalcogenide TlBiSe2

classification cond-mat.mes-hall cond-mat.str-el
keywords topologicaltlbise2bandsurfacebulkdirectenergyevidence
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We have performed high-resolution angle-resolved photoemission spectroscopy on TlBiSe2, which is a member of the ternary chalcogenides theoretically proposed as candidates for a new class of three-dimensional topological insulators. By measuring the energy band dispersions over the entire surface Brillouin zone, we found a direct evidence for a non-trivial surface metallic state showing a X-shaped energy dispersion within the bulk band gap. The present result unambiguously establishes that TlBiSe2 is a strong topological insulator with a single Dirac cone at the Brillouin-zone center. The observed bulk band gap of 0.4 eV is the largest among known topological insulators, making TlBiSe2 the most promising material for studying room-temperature topological phenomena.

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