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Efficient Site-specific Low-energy Electron Production via Interatomic Coulombic Decay Following Resonant Auger Decay

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arxiv 1303.6395 v1 pith:4UBZI6KG submitted 2013-03-26 physics.chem-ph physics.atm-clus

Efficient Site-specific Low-energy Electron Production via Interatomic Coulombic Decay Following Resonant Auger Decay

classification physics.chem-ph physics.atm-clus
keywords decayresonantaugercoulombicefficientinteratomicargonatoms
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We identified interatomic Coulombic decay (ICD) channels in argon dimers after spectator-type resonant Auger decay $2p^{-1}~3d \to 3p^{-2}3d, 4d$ in one of the atoms, using momentum resolved electron-ion-ion coincidence. The results illustrate that the resonant core excitation is a very efficient way of producing slow electrons at a specific site, which may cause localized radiation damage. We find also that ICD rate for $3p^{-2}4d$ is significantly lower than that for $3p^{-2}3d$.

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