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Three Dimensional Spin Web: A New Magnetic Lattice in Cu3TeO6

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arxiv cond-mat/0507684 v1 pith:G4PESNY3 submitted 2005-07-28 cond-mat.str-el

Three Dimensional Spin Web: A New Magnetic Lattice in Cu3TeO6

M. Herak , H. Berger , M. Prester , M. Miljak , I. Zivkovic , O. Milat , D. Drobac , S. Popovic
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O. Zaharko
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classification cond-mat.str-el
keywords magneticcu3teo6spindimensionalhexagonslatticepropertiessusceptibility
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We report on magnetic properties of cubic compound Cu3TeO6 studied by $ac$ and $dc$ susceptibility and neutron powder diffraction for the first time. A novel magnetic lattice, three dimensional spin web, composed of almost planar regular hexagons of Cu2+, S =1/2 spins, defines the properties of Cu3TeO6. The behavior of the magnetic susceptibility in the paramagnetic state at approximately 170 K is suggestive for a competition between local anisotropies of Cu2+ hexagons. The resulting frustration is weaker than the antiferromagnetic nearest-neighbor interaction which leads to a collinear (or slightly canted) spin arrangement (k=0,0,0) and formation of magnetic domains below TN=61 K.

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