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Magnetic ground state and perturbations of the distorted kagome Ising metal TmAgGe

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arxiv 2306.09867 v1 pith:IXM3PUKF submitted 2023-06-16 cond-mat.str-el

Magnetic ground state and perturbations of the distorted kagome Ising metal TmAgGe

classification cond-mat.str-el
keywords magneticcrystaldistortedkagomedetermineexchangeexperimentalground
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We present the magnetic orders and excitations of the distorted kagome intermetallic magnet TmAgGe. Using neutron single crystal diffraction we identify the propagation vectors $\bf{k}$ = (1/2 0 0) and $\bf{k}$ = (0 0 0) and determine the magnetic structures of the zero-field and magnetic field-induced phases for $H$ along the $a$ and [-1 1 0] crystal directions. We determine the experimental magnetic field-temperature ($H$, $T$)-phase diagram and reproduce it by Monte-Carlo simulations of an effective spin exchange Hamiltonian for one distorted kagome layer. Our model includes a strong axial single-ion anisotropy and significantly smaller exchange couplings which span up to the third-nearest neighbours within the layer. Single crystal inelastic neutron scattering (INS) measurements reveal an almost flat, only weakly dispersive mode around 7 meV that we use alongside bulk magnetization data to deduce the crystal-electric field (CEF) scheme for the Tm$^{3+}$ ions. Random phase approximation (RPA) calculations based on the determined CEF wave functions of the two lowest quasi-doublets enable an estimation of the interlayer coupling that is compatible with the experimental INS spectra. No evidence for low-energy spin waves associated to the magnetic order was found, which is consistent with the strongly Ising nature of the ground state.

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