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Remarkable magnetostructural coupling around the magnetic transition in CeCo_(0.85)Fe_(0.15)Si

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arxiv 1604.03985 v1 pith:LQYPNKF7 submitted 2016-04-13 cond-mat.str-el

Remarkable magnetostructural coupling around the magnetic transition in CeCo_(0.85)Fe_(0.15)Si

classification cond-mat.str-el
keywords magnetictransitioncecoexpansionmagnetostrictionresistivitytailthermal
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We report a detailed study of the magnetic properties of CeCo$_{0.85}$Fe$_{0.15}$Si under high magnetic fields (up to 16 Tesla) measuring different physical properties such as specific heat, magnetization, electrical resistivity, thermal expansion and magnetostriction. CeCo$_{0.85}$Fe$_{0.15}$Si becomes antiferromagnetic at $T_N \approx$ 6.7 K. However, a broad tail (onset at $T_X \approx$ 13 K) in the specific heat precedes that second order transition. This tail is also observed in the temperature derivative of the resistivity. However, it is particularly noticeable in the thermal expansion coefficient where it takes the form of a large bump centered at $T_X$. A high magnetic field practically washes out that tail in the resistivity. But surprisingly, the bump in the thermal expansion becomes a well pronounced peak fully split from the magnetic transition at $T_N$. Concurrently, the magnetoresistance also switches from negative to positive just below $T_X$. The magnetostriction is considerable and irreversible at low temperature ($\frac {\Delta L}{L} \left(16 T\right) \sim$ 4$\times$10$^{-4}$ at 2 K) when the magnetic interactions dominate. A broad jump in the field dependence of the magnetostriction observed at low $T$ may be the signature of a weak ongoing metamagnetic transition. Taking altogether, the results indicate the importance of the lattice effects in the development of the magnetic order in these alloys.

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