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Paramagnetic spin excitations in insulating Rb_(0.8)Fe_(1.6)Se₂

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arxiv 1211.7328 v1 pith:S3WNTUPP submitted 2012-11-30 cond-mat.supr-con cond-mat.str-el

Paramagnetic spin excitations in insulating Rb_(0.8)Fe_(1.6)Se₂

classification cond-mat.supr-con cond-mat.str-el
keywords spinexcitationsparamagnetictemperaturebecomeinsulatingironwarming
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We use neutron scattering to study temperature dependent spin excitations in insulating antiferromagnetic (AF) Rb$_{0.8}$Fe$_{1.6}$Se$_2$. In the low-temperature AF state, spin waves can be accurately described by a local moment Heisenberg Hamiltonian. On warming to around the Neel temperature of T_N=500$ K, low-energy (E<30meV) paramagnetic spin excitations form Lorentzian-like quasielastic peaks centered at the AF wave vectors associated with spin waves, while high-energy (E>50meV) spin excitations become heavily damped. Upon further warming to above the structural distortion temperature of T_s=524K, the entire paramagnetic excitations become overdamped. These results suggest that AF Rb$_{0.8}$Fe$_{1.6}$Se$_2$ is not a copper-oxide-like Mott insulator, and has less electron correlations compared with metallic iron pnictides and iron chalcogenides.

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