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Ising versus XY anisotropy in frustrated R₂Ti₂O₇ compounds as seen by polarized neutrons

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arxiv 0904.4440 v1 pith:Z3AL3DL4 submitted 2009-04-28 cond-mat.str-el

Ising versus XY anisotropy in frustrated R₂Ti₂O₇ compounds as seen by polarized neutrons

classification cond-mat.str-el
keywords fieldanisotropycompoundsinducedparallelperppolarizedtensor
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We studied the field induced magnetic order in R$_{2}$Ti$_{2}$O$_7$ pyrochlore compounds with either uniaxial (R=Ho, Tb) or planar (R=Er, Yb) anisotropy, by polarized neutron diffraction. The determination of the local susceptibility tensor \{$\chi_\parallel,\chi_\perp$\} provides a universal description of the field induced structures in the paramagnetic phase (2-270 K), whatever the field value (1-7 T) and direction. Comparison of the thermal variations of $\chi_\parallel$ and $\chi_\perp$ with calculations using the rare earth crystal field shows that exchange and dipolar interactions must be taken into account. We determine the molecular field tensor in each case and show that it can be strongly anisotropic.

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