First Energy and Angle differential Measurements of e^+e^- -pairs emitted by Internal Pair Conversion of excited Heavy Nuclei

We present the first energy and angle resolved measurements of e+e- pairs emitted from heavy nuclei (Z>=40) at rest by internal pair conversion (IPC) of transitions with energies of less than 2MeV as well as recent theoretical results using the DWBA method, which takes full account of relativistic effects, magnetic substates and finite size of the nucleus. The 1.76MeV E0 transition in Zr90 (Sr source) and the 1.77MeV M1 transition in Pb207 (Bi source) have been investigated experimentally using the essentially improved set-up at the double-ORANGE beta-spectrometer of GSI. The measurements prove the capability of the setup to cleanly identify the IPC pairs in the presence of five orders of magnitude higher beta- and gamma background from the same source and to yield essentially background-free sum spectra despite the large background. Using the ability of the ORANGE setup to directly determine the opening angle of the e+e- pairs, the angular correlation of the emitted pairs was measured. In the Zr90 case the correlation could be deduced for a wide range of energy differences of the pairs. The Zr90 results are in good agreement with recent theory. The angular correlation deduced for the M1 transition in Pb207 is in strong disagreement with theoretical predictions derived within the Born approximation and shows almost isotropic character. This is again in agreement with the new theoretical results.